Switching of the electron-phonon interaction in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mn>1</mml:mn><mml:mi>T</mml:mi></mml:mrow><mml:mtext>?</mml:mtext><mml:msub><mml:mrow><mml:mi>VSe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math> assisted by hot carriers
نویسندگان
چکیده
We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states three-dimensional charge density wave material 1$T$-VSe$_2$. Ultrafast snapshots of light-induced hot carrier dynamics non-equilibrium quasiparticle spectral function are collected using time- angle-resolved photoemission spectroscopy. The temperature time-dependent self-energy extracted from function, revealing that incoherent electron-phonon interactions heat lattice above critical on a timescale $(200 \pm 40)$~fs. Density functional perturbation theory calculations establish presence carriers alters overall phonon dispersion quenches efficient low-energy acoustic scattering channels, which results new quasi-equilibrium state is experimentally observed.
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ژورنال
عنوان ژورنال: Physical Review B
سال: 2021
ISSN: ['1098-0121', '1550-235X', '1538-4489']
DOI: https://doi.org/10.1103/physrevb.103.l241108